Inelastic decay of electrons in Shockley-type metal-organic interface states

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Inelastic decay of electrons in Shockley-type metal-organic interface states

S. S. Tsirkin,1,2,3 N. L. Zaitsev,4 I. A. Nechaev,1,2,3,5 R. Tonner,4 U. Höfer,1,4 and E. V. Chulkov1,2,3,5,6 1Donostia International Physics Center (DIPC), 20018 San Sebastián/Donostia, Basque Country, Spain 2Tomsk State University, 634050, Tomsk, Russia 3Saint Petersburg State University, Saint Petersburg, 198504, Russia 4Philipps-Universität Marburg, D-35032, Marburg, Germany 5Centro de Fı́si...

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The emergence of an organic/metal interface state is studied for the interface between 3,4,9,10-perylene-tetracarboxylic acid dianhydride (PTCDA) and Ag(100) by means of time- and angle-resolved two-photon photoemission and density functional theory. The interface state is located in the projected band gap of Ag(100), 2.3 eV above the Fermi level, and has an electron lifetime in the 10 fs range...

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ژورنال

عنوان ژورنال: Physical Review B

سال: 2015

ISSN: 1098-0121,1550-235X

DOI: 10.1103/physrevb.92.235434